PROBLEM TO BE SOLVED: To provide an electrode unit, a head set, and a paste agent application method that can easily stabilize an application amount of a paste agent applied to an electrode surface.SOLUTION: An electrode unit 1 includes: an electrode body 3 having an electrode surface 30 brought into contact with a human body through a paste agent 2 for measuring a biological signal of the human body; and a regulation member 5 for forming an application region A1 to which the paste agent 2 is applied by being located surrounding the electrode surface 30 when viewed in a second direction D2 opposite to a first direction D1 that the electrode surface 30 is oriented. The end surface 50 in the first direction D1 of the regulation member 5 is positioned higher than the electrode surface 30. The head set includes the electrode unit 1 and a frame mounted on the head of the human body, to which the electrode unit 1 is attached. In a paste agent application method, the paste agent 2 is applied to the electrode surface 30 so as to fill the application region A1 surrounded by the regulation member 5 of the electrode unit 1.SELECTED DRAWING: Figure 1COPYRIGHT: (C)2020,JPO&INPIT【課題】電極表面に塗布するペースト剤の塗布量が安定しやすい、電極ユニット、ヘッドセット及び、ペースト剤の塗布方法を提案する。【解決手段】電極ユニット1は、人体の生体信号を計測するために、ペースト剤2を介して人体に当てられる電極表面30を有する電極体3と、電極表面30が向く第一の向きD1とは反対の第二の向きD2に見て、電極表面30を囲んで位置することで、ペースト剤2が塗布される塗布領域A1を形成する規定部材5を備える。規定部材5は、第一の向きD1の端面50が電極表面30よりも高く位置する。ヘッドセットは、電極ユニット1と、電極ユニット1が取り付けられ、人体の頭部に装着されるフレームを備える。ペースト剤の塗布方法は、電極ユニット1の規定部材5で囲まれる塗布領域A1を埋めるように、電極表面30にペースト剤2を塗布する。【選択図】図1