A multi-layered ice brick and mold thereof is disclosed in the present invention. In an embodiment, a multi-layered ice brick includes a plurality of ice. The plurality of ice are formed by a plurality of molds so that the plurality of ice forms the multi-layered ice brick. The plurality of ice include: a first ice being formed by injecting a first solution into a first mold of the plurality of molds to form the first ice at a first preset temperature and a second e ice being formed by injecting a second solution into a second mold of the plurality of molds to form the second ice at a second preset temperature. The first mold is placed within the second mold. After the first mold forms the first ice, extracting the first mold from the plurality of mold, and using the second mold to form the second ice.一實施例提供了一種多層次冰磚與其模具,一種多層次冰磚,包含:複數個冰層,該複數個冰層由複數個模具成型,且該複數個冰層係成型於該複數個模具中,該複數個冰層形成該多層次冰磚,其中該複數個冰層,包含:一第一冰層,係由該複數個模具中之一第一模具注入一第一溶液,於一第一預設溫度成型該第一冰層;以及一第二冰層,係由該複數個模具中之一第二模具注入一第二溶液,於一第二預設溫度成型該第二冰層;其中,該第一模具置於該第二模具內,該第一模具成型該第一冰層後,於該複數個模具中抽出該第一模具,再利用該第二模具成型該第二冰層。100‧‧‧多層冰磚模具101a‧‧‧拉把101‧‧‧小圓形第一模具102‧‧‧大圓形第二模具