Disclosed is a method for producing a tocotrienol composition of concentrated tocotrienol, said tocotrienol composition containing tocotrienol and 1% by weight or less of tocopherol relative to the tocotrienol. The method for producing a tocotrienol composition of concentrated tocotrienol comprises a step wherein a starting material, which is selected from among (1) coconut palm oil, (2) a reaction product that is obtained by transesterification of coconut palm oil and a lower alcohol, and (3) a distillation residue of a reaction product that is obtained by transesterification of coconut palm oil and a lower alcohol, is subjected to an adsorption treatment with an anion exchange resin having a 2-hydroxyethyl dimethylammonium group.