A tooth sensitivity treatment composition is disclosed. The composition includes a compound of Formula IM1-A-M2-B-M3 (I)wherein: M1 and M3 are, independently, a monovalent or divalent metal; M2 is a polyvalent metal or metal oxide; and A and B are, independently, selected from the group consisting of C2-C6 diacids, triacids, and tetraacids. Methods for treating tooth sensitivity are also disclosed.