The present disclosure provides a dual-nuclear radio frequency (RF) coil device, including a first RF coil and a second RF coil. The first RF coil is a loop structure and includes at least one adjustment capacitor, the first RF coil is configured to generate a first magnetic field, and a direction of a primary magnetic field of the first magnetic field is a first direction. The second RF coil includes an electric dipole and a tuning and matching circuit connected between two conductors of the electric dipole. The second RF coil is configured to generate a second magnetic field and a direction of a primary magnetic field of the second magnetic field is a second direction; the electric dipole is disposed in a center line of the first RF coil and an insulating layer is disposed between the electric dipole and the first RF coil; and the first direction is perpendicular to the second direction. The present disclosure further provides a dual-nuclear RF coil array device.